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Spectroscopic Study of the Hydration Equilibria and Water Exchange Dynamics of ...
Yerly, Fabrice; Dunand, Frank A.; Tóth, Éva; Figueirinha, Artur; Kovács, Zoltán; Sherry, A. Dean; Geraldes, Carlos F. G. C.; Merbach, André E.The hydration state of a series of [Ln(DO2A)(H2O)n]+ complexes in aqueous solution at pH = 6.4-7.0 was studied by measuring the lanthanide-induced 17O shifts (LIS) of water [Ln includes elements from Ce to Yb; DO2A = 1,7-bis(carboxymethyl)-1,4,7,10-tetraazacyclododecane]. Their contact contribution, obtained from Reilley plots, indicated a decrease in the inner-sphere water coordination number of the [Ln(DO2A)(...
Data: 2000
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Origem: Estudo Geral - Universidade de Coimbra
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